LOL, Tosk from DS9's "Captive Pursuit" was a great character, if only for one episode. Still, he had a few great lines, such as:
"I am sorry I have no vices for you to exploit."
Garak and Bashir's interactions were always fantastic:
"Really, Doctor. Must we always play this game? I'm no more a spy than you are-"
"A doctor."
And the few Garak and Odo interactions:
"I see I'm going to have to add the word pickpocket to your resume." - Odo
"It's only a hobby." -Garak
Voyager also had lots of nice one-liners and quips:
"It appears we have lost our sex appeal, Captain" - Tuvok
"Do you know what a Vulcan mind meld is?" - Tuvok
"It's that thing where you grab someone's head..." - Crewman Suder
"You're on your way to being normal -- although I'm not sure how normal applies to a species who suppress all their emotions" - The Doctor
"Mr. Kim, we're Starfleet officers. Weird is part of the job" - Janeway
(Man, she really nailed that on the head!)
"Ever since my first day on the job as a Starfleet Captian, I swore I'd never let myself get caught in one of these Godforsaken paradoxes. The past is the future, the future is the past, it all gives me a headache." - Janeway
"We need to talk about this...I think we need to define some paramaters...about us." -- Janeway
"I'm not sure I can...define peramaters. But I can tell you a story, an acient legend among my people. Its about an angry warrior who lived his life in conflict with the rest of his tribe, a man who couldn't find peace even with the help of his spirit guide. For years he stuggled with his discontent, but the only satisfaction he ever got came when he was in battle. This made him a hero among his tribe, but the warrior still longed for peace within himself. One day he and his war party were captured by a neighboring tribe, lead by a woman warrior. She called on him to join her, because her tribe was too small and weak to defend itself from all its enimies. The woman warrior was brave, and beautiful, and very wise. The angry warrior swore to himself that he would stay by her side, doing whatever he could to make her burden lighter. From that point on her needs would come first; and in that way, the warrior began to know the true meaning of peace." -- Chakotay
"Is that really an ancient legend?" -- Janeway
"No...but that made it easier to say." -- Chakotay
And TNG, of course, had Data:
"They were just sucked into space" -- Riker
"Blown, sir" -- Data
"Sorry, Data" -- Riker
"Common mistake, sir" -- Data
[after they kiss] "What were you just thinking?" -- Jenna
"In that particular moment, I was reconfiguring the warp field parameters, analyzing the collected works of Charles Dickens, calculating the maximum pressure I could safely apply to your lips, considering a new food supplement for Spot..." -- Data
"I'm glad I was in there somewhere" -- Jenna
"You are capable of great sadism and cruelty. Interesting, no redeeming
qualities." -Data
"I hope I did not do anything unbecoming a Starfleet officer."
"Does wrestling a Klingon targ ring a bell?" -Riker
"Did I win?"
Ah, they're all so good...
"I am sorry I have no vices for you to exploit."
Garak and Bashir's interactions were always fantastic:
"Really, Doctor. Must we always play this game? I'm no more a spy than you are-"
"A doctor."
And the few Garak and Odo interactions:
"I see I'm going to have to add the word pickpocket to your resume." - Odo
"It's only a hobby." -Garak
Voyager also had lots of nice one-liners and quips:
"It appears we have lost our sex appeal, Captain" - Tuvok
"Do you know what a Vulcan mind meld is?" - Tuvok
"It's that thing where you grab someone's head..." - Crewman Suder
"You're on your way to being normal -- although I'm not sure how normal applies to a species who suppress all their emotions" - The Doctor
"Mr. Kim, we're Starfleet officers. Weird is part of the job" - Janeway
(Man, she really nailed that on the head!)
"Ever since my first day on the job as a Starfleet Captian, I swore I'd never let myself get caught in one of these Godforsaken paradoxes. The past is the future, the future is the past, it all gives me a headache." - Janeway
"We need to talk about this...I think we need to define some paramaters...about us." -- Janeway
"I'm not sure I can...define peramaters. But I can tell you a story, an acient legend among my people. Its about an angry warrior who lived his life in conflict with the rest of his tribe, a man who couldn't find peace even with the help of his spirit guide. For years he stuggled with his discontent, but the only satisfaction he ever got came when he was in battle. This made him a hero among his tribe, but the warrior still longed for peace within himself. One day he and his war party were captured by a neighboring tribe, lead by a woman warrior. She called on him to join her, because her tribe was too small and weak to defend itself from all its enimies. The woman warrior was brave, and beautiful, and very wise. The angry warrior swore to himself that he would stay by her side, doing whatever he could to make her burden lighter. From that point on her needs would come first; and in that way, the warrior began to know the true meaning of peace." -- Chakotay
"Is that really an ancient legend?" -- Janeway
"No...but that made it easier to say." -- Chakotay
And TNG, of course, had Data:
"They were just sucked into space" -- Riker
"Blown, sir" -- Data
"Sorry, Data" -- Riker
"Common mistake, sir" -- Data
[after they kiss] "What were you just thinking?" -- Jenna
"In that particular moment, I was reconfiguring the warp field parameters, analyzing the collected works of Charles Dickens, calculating the maximum pressure I could safely apply to your lips, considering a new food supplement for Spot..." -- Data
"I'm glad I was in there somewhere" -- Jenna
"You are capable of great sadism and cruelty. Interesting, no redeeming
qualities." -Data
"I hope I did not do anything unbecoming a Starfleet officer."
"Does wrestling a Klingon targ ring a bell?" -Riker
"Did I win?"
Ah, they're all so good...
SAM & JACK 4EVER!!
thats so funny
and Spudster made another neat one 
Dr. Lee RULES!
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